Download e-book for kindle: Advances in Organometallic Chemistry, Vol. 15 by F.G.A. Stone, Robert West

By F.G.A. Stone, Robert West

ISBN-10: 0120311151

ISBN-13: 9780120311156

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C. Polyenes . . . . . . . . . IV. Insertion Reactions of Metal Atoms . . . . . A. Carbon-Halogen Compounds . . . . . B. Other Insertion and Oxidation Reactions . . . . V. Discussion . . . . . . . . . A. Yields of Products . . . . . . . B. Comparison of Metal Atom with Other Synthetic Methods . VI . Appendix: Tables of Metal Vapor Reactions . . . . References . . . . . . . . . I. 53 54 55 59 59 63 63 66 66 72 76 78 78 83 84 84 86 87 108 I INTRODUCTION The first report of the preparation of organometallic compounds by direct reaction between metals atoms and organic ligands came in 1969 (127).

R-level (see Table IV). Therefore, if the stability of the metal-olefin complexes is correlated simply with the energy of the fluoroolefin p*-level in accordance with the simple perturbation theory analysis. then their stability constants are grossly underestimated (see Fig. 13). Tolman has suggested that this apparent failure of the perturbation approach arises from using electronic spectral data appropriate for the planar D2,, olefin. r*-orbitals of the fluorinated olefins may drop sufficiently to allow a strong interaction with the occupied metal orbitals.

Armstrong, D. , Perkins, P. , and Stewart, J. , J . Chem. , Dalton Trans. 3674 (1971). 8. Armstrong, D. , Perkins, P. , and Stewart, J. J. , J . Chem. , Dalton Trans. 1972 (1972). 9. Ashley-Smith, J . , Johnson, B. F. , J. Chem. , Dalton Trans. 128 (1974). 10. Ballhausen, C. ” McGraw-Hill, New York, 1972. 11. Ballhausen, C. , Int. J . Quantum. , Symp. 5, 373 (1971). 12. Ballhausen, C. , and Dahl, J. , Acta Chem. Scund. 15, 1333 (1961). 13. Ballhausen, C. , and Gray, H. ” Benjamin, New York, 1964.

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Advances in Organometallic Chemistry, Vol. 15 by F.G.A. Stone, Robert West


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